Foundation is probably where you will see the most benefits from switching to an organic product. Since your skin absorbs the materials you put on it, the lighter organic makeup will be more breathable on your skin and will not irritate your skin with regular use like other makeup.
Check out these products from some top makeup brands.
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Eyeliner & Mascara
Although it's probably covering the least amount of surface area on your face, don't forget to keep it organic when it comes to your eyeliner and mascara.